The answer is without doubt, and is consistent all year, whether during a Free Communication Weekend or not:

The day of the week that eHarmony gets tons and tons of traffic is Monday, followed by Sunday or Tuesday. Monday night, we think, is the best time to expect a quick reply to your messages to matches.
The worst days of the week to use eHarmony is Friday and Saturday.
Why can we say this? Because our traffic follows eHarmony traffic exactly. Our promo codes poll votes, keyword searches, hits and pageviews have the same “day of week” trend.

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